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Modeling of coal swelling induced by water vapor adsorption

Zhejun PAN

《化学科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 94-103 doi: 10.1007/s11705-011-1172-2

摘要： Gas adsorption-induced coal swelling is a well-know phenomenon. Coal swelling or shrinkage by adsorption or desorption of water vapor has not been well understood but has significant implications on gas drainage process for underground coal mining and for primary and enhanced coalbed methane production. Decreased matrix moisture content leads to coal shrinkage and thus the change of cleat porosity and permeability under reservoir conditions. Unlike gas adsorption in coal which usually forms a single layer of adsorbed molecules, water vapor adsorption in the coal micropores forms multilayer of adsorbed molecules. In this work, a model has been developed to describe the coal swelling strain with respect to the amount of moisture intake by the coal matrix. The model extended an energy balance approach for gas adsorption-induced coal swelling to water vapor adsorption-induced coal swelling, assuming that only the first layer of adsorbed molecules of the multilayer adsorption changes the surface energy, which thus causes coal to swell. The model is applied to describe the experimental swelling strain data measured on an Australian coal. The results show good agreement between the model and the experimental data.

关键词： multilayer adsorption     vapour pressure     coal shrinkage     relative humidity     permeability    

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FEM-based strain analysis study for multilayer sheet forming process

Rongjing ZHANG,Lihui LANG,Rizwan ZAFAR

《机械工程前沿（英文）》 2015年 第10卷 第4期   页码 373-379 doi: 10.1007/s11465-015-0371-9

摘要：

Fiber metal laminates have many advantages over traditional laminates (e.g., any type of fiber and resin material can be placed anywhere between the metallic layers without risk of failure of the composite fabric sheets). Furthermore, the process requirements to strictly control the temperature and punch force in fiber metal laminates are also less stringent than those in traditional laminates. To further explore the novel method, this study conducts a finite element method-based (FEM-based) strain analysis on multilayer blanks by using the 3A method. Different forming modes such as wrinkling and fracture are discussed by using experimental and numerical studies. Hydroforming is used for multilayer forming. The Barlat 2000 yield criteria and DYNAFORM/LS-DYNA are used for the simulations. Optimal process parameters are determined on the basis of fixed die-binder gap and variable cavity pressure. The results of this study will enhance the knowledge on the mechanics of multilayer structures formed by using the 3A method and expand its commercial applications.

关键词： finite element method (FEM)     strain analysis     multilayer sheet forming    

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Mechanical properties and microstructure of multilayer graphene oxide cement mortar

《结构与土木工程前沿（英文）》 2021年 第15卷 第4期   页码 1058-1070 doi: 10.1007/s11709-021-0747-3

摘要： This study reports on the effects of multilayer graphene oxide (MGO) on compressive strength, flexural strength, and microstructure of cement mortar. The cement mortar was prepared with type P. II. 52.5 Portland cement, standard sand, and MGO. Four mixes were prepared with inclusion of MGO (0%, 0.02%, 0.04%, and 0.06% by weight of cement). The testing result shows that the compressive of GO-cement mortar increased by 4.84%–13.42%, and the flexural strength increased by 4.37%–8.28% at 3 d. GO-cement mortar’s compressive strength and flexural strength at 7 d increased by 3.84%–12.08% and 2.54%–13.43%, respectively. MGO made little contribution to the increases of compressive strength and flexural strength of cement mortar at 28 d. The results of X-ray diffraction (XRD), scanning electron microscope (SEM), and nitrogen (N2) adsorption/desorption tests show that the types of hydration products and crystal grain size did not change after adding MGO. Still, it can help to improve the microstructure of the cement mortar via regulating hydration products and can provide more condensed cores to accelerate hydration. Furthermore, the regulating action of MGO for the microstructure of cement mortar at an early age was better than that at 28 d.

关键词： graphene oxide     cement     mortar     mechanical properties     microstructure    

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Eddy current measurement of the thickness of top Cu film of the multilayer interconnects in the integrated

Zilian QU,Yonggang MENG,Qian ZHAO

《机械工程前沿（英文）》 2015年 第10卷 第1期   页码 1-6 doi: 10.1007/s11465-015-0325-2

摘要：

This paper proposes a new eddy current method, named equivalent unit method (EUM), for the thickness measurement of the top copper film of multilayer interconnects in the chemical mechanical polishing (CMP) process, which is an important step in the integrated circuit (IC) manufacturing. The influence of the underneath circuit layers on the eddy current is modeled and treated as an equivalent film thickness. By subtracting this equivalent film component, the accuracy of the thickness measurement of the top copper layer with an eddy current sensor is improved and the absolute error is 3 nm for sampler measurement.

关键词： CMP     eddy current     multilayer wafer     Cu interconnects     equivalent unit    

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Experimental verification of the interface wave method to detect interlaminar damage of a metal multilayer

Bing LI,Xu GENG,Tong LU,Lei QIANG,Minghang LI

《机械工程前沿（英文）》 2015年 第10卷 第4期   页码 380-391 doi: 10.1007/s11465-015-0365-7

摘要：

The interface wave traveling along the boundary of two materials has been studied for nearly a century. However, experiments, engineering applications, and interface wave applications to the non-destructive inspection of interlaminar composite have developed slowly. In this research, an experiment that applies Stoneley waves (a type of interfacial wave between two solid half-spaces) is implemented to detect the damage in a multilayer structure. The feasibility of this method is also verified. First, the wave velocity and wave structure of Stoneley waves at a perfectly bonded aluminum-steel interface are obtained by solving the Stoneley wave dispersion equation of two elastic half-spaces. Thereafter, an experiment is conducted to measure the Stoneley wave velocity of an aluminum-steel laminated beam and to locate interlaminar cracks by referring to the Stoneley wave velocity and echo wave time. Results indicate that the location error is less than 2%. Therefore, Stoneley waves show great potential as a non-destructive inspection method of a multilayer structure.

关键词： crack localization     interface waves     Stoneley waves     interlaminar damage     multilayer structure    

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Experimental research on the multilayer compartmental particle damper and its application methods on

Zhenyuan LUO, Weiming YAN, Weibing XU, Qinfei ZHENG, Baoshun WANG

《结构与土木工程前沿（英文）》 2019年 第13卷 第4期   页码 751-766 doi: 10.1007/s11709-018-0509-z

摘要： Particle damping technology has attracted extensive research and engineering application interest in the field of vibration control due to its prominent advantages, including wide working frequency bands, ease of installation, longer durability and insensitivity to extreme temperatures. To introduce particle damping technology to long-period structure seismic control, a novel multilayer compartmental particle damper (MCPD) was proposed, and a 1/20 scale test model of a typical long-period self-anchored suspension bridge with a single tower was designed and fabricated. The model was subjected to a series of shaking table tests with and without the MCPD. The results showed that the seismic responses of the flexible or semi-flexible bridge towers of long-period bridges influence the seismic responses of the main beam. The MCPD can be conveniently installed on the main beam and bridge tower and can effectively reduce the longitudinal peak displacement and the root mean square acceleration of the main beam and tower. In addition, no particle accumulation was observed during the tests. A well-designed MCPD can achieve significant damping for long-period structures under seismic excitations of different intensities. These results indicate that the application of MCPDs for seismic control of single-tower self-anchored suspension bridges and other long-period structures is viable.

关键词： energy dissipation devices     multilayer compartmental particle damper     self-anchored suspension bridges     shaking tables test     long-period structure     seismic control    

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Contributions of adsorption, bioreduction and desorption to uranium immobilization by extracellular polymeric

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1707-z

摘要：

● EPS immobilizes U(VI) via adsorption, bioreduction and desorption.

关键词： Adsorption     Bioreduction     Desorption     Kinetics     Isotherm     Uranium    

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Polypropylene microplastics alter the cadmium adsorption capacity on different soil solid fractions

《环境科学与工程前沿（英文）》 2022年 第16卷 第1期   页码 3-3 doi: 10.1007/s11783-021-1437-z

摘要：

Microplastics (MPs) are widely present in a variety of environmental media and have attracted more and more attention worldwide. However, the effect of MPs on the interaction between heavy metals and soil, especially in soil solid fraction level, is not well understood. In this study, batch experiments were performed to investigate the adsorption characteristics of Cd in bulk soil and three soil solid fractions (i.e. particulate organo matter (POM), organic-mineral compounds (OMC), and mineral) with or without polypropylene (PP) MPs.

关键词： Polypropylene microplastics     Cadmium     Adsorption     POM     OMC     Mineral    

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Cesium removal from radioactive wastewater by adsorption and membrane technology

《环境科学与工程前沿（英文）》 2023年 第18卷 第3期 doi: 10.1007/s11783-024-1798-1

摘要：

● Removal of cesium from radioactive wastewater is still a challenging.

关键词： Cesium     Adsorption     Membrane separation     Advanced liquid processing system     Fukushima nuclear accident    

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Dual-functional sites for synergistic adsorption of Cr(VI) and Sb(V) by polyaniline-TiO hydrate: Adsorption

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1526-7

摘要：

• PANI/Ti(OH)n(4–n)+ exhibited excellent adsorption capacity and reusability.

关键词： Polyaniline/TiO2     Chromium     Antimony     Adsorption     Desorption     Mechanism    

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Kinetics and thermodynamics of the phosphine adsorption on the modified activated carbon

Bingnan REN

《化学科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 203-208 doi: 10.1007/s11705-010-0571-0

摘要： The kinetics and the thermodynamics of phosphine (PH ) adsorption on the modified activated carbon have been explained for the adsorption process of PH . This study investigated the kinetic and thermodynamic properties of PH adsorption on the activated carbon impregnated with 5% HCl solution. The thermodynamic properties including PH adsorption isotherm and adsorption heat were separately investigated at 20°C, 70°C, 90°C. The results showed that the Freundlich-type isotherm equation described the isotherms well. The adsorption capacity increased with increasing temperature between 20°C and 70°C. Between 70°C and 90°C, the adsorption capacity decreased obviously with increasing temperature. The adsorption capacity reached the maximum at 70°C. By analyzing the results of the kinetics and the thermodynamics, we found that the adsorption of PH was dominated by physical adsorption at the lower temperature (20°C). Then with increasing temperature, chemical adsorption gradually dominated in the adsorption process. The adsorption capacity decreased at above 70°C is due to the exothermic effects in the process of adsorption.

关键词： adsorption     PH3     activated carbon     kinetics     thermodynamics    

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An adsorption study of

Lingxiao FU, Jianhua ZU, Enxi GU, Huan WANG, Linfeng HE

《能源前沿（英文）》 2020年 第14卷 第1期   页码 11-17 doi: 10.1007/s11708-019-0634-y

摘要： Nanoscale zero-valent iron (nZVI) supported on D001 resin (D001-nZVI) was synthesized for adsorption of high solubility and mobility radionuclide Tc. Re(VII), a chemical substitute for Tc, was utilized in batch experiments to investigate the feasibility and adsorption mechanism toward Tc(VII). Factors (pH, resin dose) affecting Re(VII) adsorption were studied. The high adsorption efficiency of Re(VII) at pH= 3 and the solid-liquid ratio of 20 g/L. X-ray diffraction patterns revealed the reduction of into ReO immobilized in D001-nZVI. Based on the optimum conditions of Re(VII) adsorption, the removal experiments of Tc(VII) were conducted where the adsorption efficiency of Tc(VII) can reach 94%. Column experiments showed that the Thomas model gave a good fit to the adsorption process of Re(VII) and the maximum dynamic adsorption capacity was 0.2910 mg/g.

关键词： technetium     nanoscale zero-valent iron (nZVI)     D001 resin     adsorption    

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Dialdehyde cellulose nanocrystal cross-linked chitosan foam with high adsorption capacity for removal

《化学科学与工程前沿（英文）》 2023年 第17卷 第7期   页码 853-866 doi: 10.1007/s11705-022-2256-x

摘要： The discharge of large amounts of dye-containing wastewater seriously threats the environment. Adsorbents have been adopted to remove these dyes present in the wastewater. However, the high adsorption capacity, predominant pH-responsibility, and excellent recyclability are three challenges to the development of efficient adsorbents. The poly(acryloxyethyl trimethylammonium chloride)-graft-dialdehyde cellulose nanocrystals were synthesized in our work. Subsequently, the cationic dialdehyde cellulose nanocrystal cross-linked chitosan nanocomposite foam was fabricated via freeze-drying of the hydrogel. Under the optimal ratio of the cationic dialdehyde cellulose nanocrystal/chitosan (w/w) of 12/100, the resultant foam (Foam-12) possesses excellent absorption properties, such as high porosity, high content of active sites, strong acid resistance, and high amorphous region. Then, Foam-12 was applied as an eco-friendly adsorbent to remove acid red 134 (a representative of anionic dyes) from aqueous solutions. The maximum dye adsorption capacity of 1238.1 mg∙g‒1 is achieved under the conditions of 20 mg∙L‒1 adsorbents, 100 mg∙L‒1 dye, pH 3.5, 24 h, and 25 °C. The dominant adsorption mechanism for the anionic dye adsorption is electrostatic attraction, and Foam-12 can effectively adsorb acid red 134 at pH 2.5–5.5 and be desorbed at pH 8. Its easy recovery and good reusability are verified by the repeated acid adsorption–alkaline desorption experiments.

关键词： chitosan foam     cellulose nanocrystals     acid red 134     adsorption    

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Effect of gastric fluid on adsorption and desorption of endocrine disrupting chemicals on microplastics

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1525-8

摘要：

• Effect of gastric fluid on EDCs adsorption-desorption to microplastics was evaluated.

关键词： Microplastics     Gastric fluid     Endocrine-disrupting chemicals     Adsorption     Desorption    

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Ammonia adsorption on graphene and graphene oxide: a first-principles study

Yue PENG, Junhua LI

《环境科学与工程前沿（英文）》 2013年 第7卷 第3期   页码 403-411 doi: 10.1007/s11783-013-0491-6

摘要： Motivated by the recent realization of graphene sensor to detect gas molecules that are harmful to the environment, the ammonia adsorption on graphene or graphene oxide (GO) was investigated using first-principles calculation. The optimal adsorption and orientation of the NH molecules on the graphene surfaces were determined, and the adsorption energies ( ) as well as the Mulliken charge transfers of NH were calculated. The for the graphene are small and seem to be independent of the sites and orientations. The surface epoxy or hydroxyl groups can promote the adsorption of NH on the GO; the enhancement of the for the hydroxyl groups is greater than that for the epoxy groups on the surface. The charge transfers from the molecule to the surfaces also exhibit the same trend. The Br?nsted acid sites and Lewis acid sites could stably exist on the GO with surface hydroxyl groups and on the basal, respectively.

关键词： graphene oxide     first-principles calculations     NH3 adsorption    

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标题 作者 时间 类型 操作

Modeling of coal swelling induced by water vapor adsorption

Zhejun PAN

期刊论文

FEM-based strain analysis study for multilayer sheet forming process

Rongjing ZHANG,Lihui LANG,Rizwan ZAFAR

期刊论文

Mechanical properties and microstructure of multilayer graphene oxide cement mortar

期刊论文

Eddy current measurement of the thickness of top Cu film of the multilayer interconnects in the integrated

Zilian QU,Yonggang MENG,Qian ZHAO

期刊论文

Experimental verification of the interface wave method to detect interlaminar damage of a metal multilayer

Bing LI,Xu GENG,Tong LU,Lei QIANG,Minghang LI

期刊论文

Experimental research on the multilayer compartmental particle damper and its application methods on

Zhenyuan LUO, Weiming YAN, Weibing XU, Qinfei ZHENG, Baoshun WANG

期刊论文

Contributions of adsorption, bioreduction and desorption to uranium immobilization by extracellular polymeric

期刊论文

Polypropylene microplastics alter the cadmium adsorption capacity on different soil solid fractions

期刊论文

Cesium removal from radioactive wastewater by adsorption and membrane technology

期刊论文

Dual-functional sites for synergistic adsorption of Cr(VI) and Sb(V) by polyaniline-TiO hydrate: Adsorption

期刊论文

Kinetics and thermodynamics of the phosphine adsorption on the modified activated carbon

Bingnan REN

期刊论文

An adsorption study of

Lingxiao FU, Jianhua ZU, Enxi GU, Huan WANG, Linfeng HE

期刊论文

Dialdehyde cellulose nanocrystal cross-linked chitosan foam with high adsorption capacity for removal

期刊论文

Effect of gastric fluid on adsorption and desorption of endocrine disrupting chemicals on microplastics

期刊论文

Ammonia adsorption on graphene and graphene oxide: a first-principles study

Yue PENG, Junhua LI

期刊论文